A finite element model for nonlinear behaviour of piezoceramics under weak electric fields M.K. Samala,∗ , P. Seshub , S. Parasharc , U. von Wagnerd , P. Hagedornc , B.K. Duttaa , H.S. Kushwahaa a Reactor Safety Division, Bhabha Atomic Research Centre, Trombay, Mumbai-400085, India b Department of Mechanical Engineering, Indian Institute of Technology Bombay, Mumbai-400076, India c Department of Applied Mechanics, Technical University of Darmstadt, 64289 Darmstadt, Germany. d Department of Applied Mechanics, Technical University of Berlin, 10587 Berlin, Germany. Abstract It has been experimentally observed that piezoceramic materials exhibit different types of nonlinearities under different combinations of electric and mechanical fields. When excited near resonance in the presence of weak e to a Duffinor such as jump phenomena and presence of superharmonics in the response spectra. There has not been much work in the litrature to model these types of nonlinearities. Some authors have developed one-dimensional models for the above phenomenon and derived closed-form solutions for the displacement response of piezo-actuators. However, the generalized three-dimensional (3-D) formulation of electric enthalpy, the variational formulation and the FEM implementation have not yet been addressed, which are the focus of this paper. In this work, these nonlinearities have been modelled in a 3-D piezoelectric continuum using higher order quadratic and cubic terms in the generalized electric enthalpy density function. The coupled nonlinear finite element equations have been derived using variational formulation. A special linearization technique for assembling the nonlinear matrices and solution of the resulting nonlinear equations has been developed. The method has been used for simulating the nonlinear frequency response of a lead zirconate titanate plate excited near its first in-plane vibration resonance frequency with sinusoidal excitations of different electric field strengths. The results have been compared with those of the experiment. Keywords: Finite element method; Piezoceramic; Nonlinear modelling; Jump phenomena 1465 1. Introduction Smart materials, especially piezoceramics, find a wide range of applications in many industries for active vibration control, shape control and health monitoring of structures [1,2]. These piezoceramics have been extensively studied in recent years for actuator and sensor applications because of their high electro-mechanical coupling coefficient. Some special classes of these actuators, known as ultrasonic transducers, are driven at resonance frequency. Depending upon the direction of polarization and direction of actuation, these can be known as axial, transverse or flexural transducers. High-power transverse piezoelectric actuators are used for ultrasonic cleaners, piezo-vibrators and machine cutters, etc. It is well known that the mechanical and electrical responses of a piezoelectric material are coupled. When the applied electric field is low and the strains are also low, the behaviour of piezoceramics is almost linear. But, it has been seen from experiments that the piezoelectric materials exhibit a wide range of nonlinear effects under both high and low electric fields when operated in the presence of high and low stress fields. The nonlinear behaviours under high and low electric fields are different in some aspects. For example, the nonlinearities observed under high electric fields are hysteresis behaviour between the electric field and strain, nonlinear relation between electric field and mechanical displacement etc. The nonlinearities observed under weak electric fields are jump phenomena (Fig. 1), dependence of resonance frequency on vibration amplitude, presence of superharmonics in the response spectra and nonlinear relationship between applied electric voltage and mechanical displacement, etc. The significant change of the displacement amplitude at a particular frequency is called a “jump phenomenon”. The frequency at which this phenomenon occurs is also different for increasing (sweep-up) and decreasing (sweepdown) frequency modes. The problem associated with piezo-actuators showing the jump phenomena can be excessive heat generation, mechanical breakdown and instability of vibration when operating in the resonant mode, etc. The different nonlinear behaviours of piezo-actuators can also affect other applications such as the active shape and vibration control of structures [3,4]. In this work, experiments have been conducted on lead zirconate titanate (PZT) plates under electric fields of varying field strengths to study these nonlinearities. The first in-plane vibration mode of the plate is being studied to observe the effect of piezoelectric nonlinearity. Based on the observed experimental Fig. 1. Jump phenomena observed in the sweepup and sweepdown frequency response behaviour of a piezo-plate. 1466 behaviour (similar to a Diffing oscillator), theoretical models have been developed for the electric enthalpy density function, which is subsequently used in Hamilton’s principle to derive governing equations for the piezo-continuum. A generalized nonlinear finite element model has been developed from the governing equations so that it can be applied to predict the actual behaviour of piezo-actuators or resonators operating in resonance mode for which closed-form solutions cannot be derived. There are many models for nonlinearities under strong electric fields (e.g., hysteresis), which are mainly based on the classical Preisach model and its modified versions [5]. However, there are very few research works existing in the literature which deal with nonlinear effects under weak electric fields. Beige and Schmidt [6] first described these nonlinear effects while conducting experiments on longitudinal vibrations of piezo-rods [6]. They modelled these nonlinearities using higher order quadratic and cubic terms in the energy expression contributed by elastic, piezoelectric and dielectric continuum. Von Wagner and Hagedorn [7] and von Wagner [8] modelled both the nonlinear d31 and d33 effects of typical PZT-based piezoceramics (i.e., PIC 181 and PIC 255) by assuming that the softening behaviour of the material is due to the nonlinear dependence of Young’s modulus and the piezoelectric coefficient on the mechanical and electrical field variables [7,8]. They derived the electric enthalpy density functions for the one-dimensional (1-D) continuum. The governing 1-D nonlinear equation was derived using variational formulation (Hamilton’s principle) and was solved using Rayleigh–Ritz method. The shape function of only one mode of vibration of the structure was used as the weighting function in this method. The discretized equation was solved for the amplitude of vibration using perturbation techniques and harmonic balance methods. The unknowns in the model, i.e., the nonlinear parameters in the constitutive relations were determined by minimizing the error between experimental and theoretical results. This was one of the first attempts to obtain closed-form solutions for simplified 1-D problems. However, when the structures to be modelled have complicated geometry, boundary condition and loading types (as in the case of machine cutters, piezo-resonators, etc.), it is no longer possible to obtain closed-form solutions for these classes of nonlinear problems. Our aim here is to formulate the generalized 3-D electric enthalpy density function. Once the electric enthalpy density function is formulated, the governing equations can be derived using variational formulation. However, one has to resort to some numerical method (e.g., FEM) to solve the system of equations. Several authors have used FEM to model various piezoelectric material systems [9–15]. However, their work is mainly directed towards modelling of the linear piezoelectric behaviour. Saravanos et al. [16] have developed a layer-wise FE model for the dynamic analysis of piezoelectric composite plates. Recently, Wang [17] has developed an FE model for static and dynamic analysis of piezoelectric bimorphs. Wang et al. [18] have studied the dynamic stability behaviour of FE models for piezo-composite plates. A generalized FE model taking into consideration of the nonlinearity of a piezo-continuum similar to a Duffing oscillator is not available in the literature. In this work, the generalized 3-D nonlinear constitutive equations for the nonlinear problem have been derived after the electric enthalpy density function had been conceived. Based on this, the FEM-based solution technique has been developed. The method has been applied to calculate the nonlinear frequency response behaviour of a PZT plate excited near its first in-plane resonance frequency for which experimental results are available. 2. Constitutive equations of the piezoelectric continuum The electric enthalpy density function H is generally used to derive the governing equations of the coupled piezoelectric continuum and for the linear piezoelectric behaviour. It is given as (IEEE 1467 standard [19]) H = 21 CijE kl Sij Skl − ekij Ek Sij − 21 Sij Ei Ej , (1) where CijE kl is the fourth-order elastic tensor under a constant electric field, ekij is the third order piezoelectric tensor, Sij is the second-order dielectric tensor, Sij is the strain tensor and Ei is the electric field vector. The stress tensor Tij and the electric displacement vector Di can be derived from H using the expressions Tij = jH /jSij and Di = −jH /jEi , respectively. It can be easily seen that the expressions for Tij and Di are coupled with the secondary field variables Sij (strain tensor) and Ei (electric field vector), respectively. Sij is expressed in terms of the mechanical displacement vector ui as Sij = (ui,j + uj,i )/2 and Ei is expressed in terms of electric potential as Ei = −,i . Keeping in mind the fact that stress and strain tensor are symmetric, H can be simplified and written in terms of second-order tensors as H = 21 CijE Si Sj − eij Ei Sj − 21 Sij Ei Ej . (2) In order to model the nonlinearities in a coupled piezoelectric medium, we propose to modify the linear electric enthalpy density function in the following way. It was experimentally observed that second- and third-order harmonics are present in the response spectra of PZT piezoceramic plates and rod geometries. The observed behaviour can be modelled using quadratic and cubic order terms in the energy terms of the two coupled mediums. Hence, the generalized expression for nonlinear electric enthalpy density function can be written as Hnonl = 21 CijE Si Sj − emi Em Si − 21 Smn Em En + 13 CijE k Si Sj Sk + 41 CijE kl Si Sj Sk Sl − 13 Smno Em En Eo ∗ ∗∗ − 41 Smnop Em En Eo Ep − 21 emij Em Si Sj − 21 emni Em En Si − 13 emij k Em Si Sj Sk ∗∗∗ ∗∗∗ − 41 emnij Em En Si Sj − 13 emnoi Em En Eo Si , (3) where the coefficients with 3 and 4 number of indices are higher order quadratic and cubic coefficients, respectively. However, this form of Hnonl is not suitable for derivation of nonlinear FEM matrices using variational formulation. Hence, the authors have envisaged a suitable matrix expression for Hnonl retaining the nonlinear terms and it is given as follows: Hnonl = 21 {S}T [C]{S} − {E}T [d][C]{S} − 21 {E}T [[T ] − [d][C][d]T ]{E} + 13 {S}T [C1 ]{S 2 } + 41 {S 2 }T [C21 ]{S 2 } + 41 {S}T [C22 ]{S 3 } − 21 {E}T [11 ]{S 2 } − 21 {E 2 }T [12 ]{S} − 13 {E}T [1 ]{E 2 } − 13 {E}T [21 ]{S 3 } − 21 {E 2 }T [22 ]{S 2 } − 13 {E 3 }T [23 ]{S} − 41 {E}T [21 ]{E 3 } − 41 {E 2 }T [22 ]{E 2 }, (4) where {S} is the strain vector, [C] is the linear elasticity matrix, [d] is the linear piezoelectric coefficient matrix, {E} is the electric field vector, [T ] is the dielectric coefficient matrix, [C1 ] is the quadratic elasticity matrix, and [C21 ] and [C22 ] are cubic elasticity matrices at a constant electric field, respectively. 1468 The superscript E (matrices at a constant electric field) for these matrices has been omitted for clarity. [11 ] and [12 ] are quadratic piezoelectric matrices, [21 ], [22 ] and [23 ] are cubic piezoelectric matrices, and [0 ] = [[T ] − [d][C][d]T ], [1 ], [21 ] and [22 ] are linear, quadratic and cubic dielectric matrices at constant strain field S, respectively. The superscript S (matrices at a constant strain field) for these matrices has been omitted for clarity. The vectors with superscripts 2 and 3 are defined as the vectors with square and cube of individual terms of the vectors. The first three terms of Hnonl correspond to the linear electric enthalpy density function. Using this expression of Hnonl , the FE matrices have been derived in the next section using variational formulation. 3. Variational formulation The dynamic equations of a piezoelectric continuum can be derived from the Hamilton principle, in which the Lagrangian and the virtual work are properly adapted to include the electrical, mechanical as well as the coupled electro-mechanical terms. The potential energy density of a piezoelectric material includes contributions from the strain energy and from the electrostatic energy. The Hamilton principle can be written as t1 t0 V L dV dt + t1 t0 W dt = 0, (5) where t0 and t1 define the time interval, L is the Lagrangian and is defined by the sum of kinetic energy Tke and electrical enthalpy density H and given as L = (Tke − H ), and W is the virtual work done by external mechanical and electrical forces. The kinetic energy is given as Tke = 21 {u̇}T {u̇}, (6) where is the mass density, {u} is the generalized displacement field and {u̇} is the generalized velocity field. The nonlinear electric enthalpy density function Hnonl is given in Eq. (4). The virtual work done by the external mechanical forces F and the applied electric charges Q for an arbitrary variation of the displacement field {u} and electrical potential {}, both satisfying the essential boundary conditions (i.e., {u} = 0 on surface As3 and {} = 0 on surface As4 ), can be written as W = {u} {FV } dV + T V {u} {FAs } dAs + {u} {FP } − T As1 T As2 dAs − Q + WD , (7) where {FV } is the applied body force vector, {FAs } is the applied surface force vector (defined on the surface As1 ), {FP } is the applied point load vector, is the electric potential, is the surface charge conferred on surface As2 , Q is the applied concentrated electric charge and WD is the work done by damping forces (we assume proportional viscous damping here). In this problem, there are no external mechanical or electrical forces except the applied electric potential at the electrodes coated to the surfaces of the piezoceramic. Now, putting the nonlinear electric enthalpy function Hnonl and kinetic 1469 energy Tke from Eqs. (4) and (6), the Hamilton’s principle becomes t1 [{u}T {ü}] dV dt − V t0 [C]{S} − [C]T [d]T {E} − [diag({S})][11 ]T {E} − 21 [12 ]T {E 2 } t1 +[diag({S})][C21 ][diag({S})]{S} + 1 [C22 ]{S 3 } + 3 [diag({S 2 })][C22 ]T {S} 4 4 {S}T − + 1 [C1 ]{S 2 } + 2 [diag({S})][C1 ]T {S} − [diag({S 2 })][ ]T {E} t0 V 21 3 3 −[diag({S})][22 ]T {E 2 } − 13 [23 ]T {E 3 } × dV dt [d][C]{S} + [0 ]{E} + 21 [11 ]{S 2 } t1 +[diag({E})][12 ]{S} + 1 [13 ]{S 2 } + 2 [diag({E})][13 ]T {E} 3 3 {E}T − 1 3 2 2 + [ ]{S } + [diag({E})][ ]{S } + [diag({E })][ ]{S} t0 V 3 21 22 23 + 41 [1 ]{E 3 } + 43 [diag({E 2 })][1 ]T {E} + [diag({E})][2 ][diag({E})]{E} × dt t1 t1 tdV 1 T T [{u} {FV }] dV dt + [{u} {FAs }] dAs dt + {u}T {FP } dt + t V t0 As1 t0 t1 t1 0t1 dAs dt − Q dt − [WD ] dt = 0, − t0 As2 t0 t0 (8) where the matrix with ‘diag’ refers to a diagonal matrix with the main diagonal terms being the terms of the vector that it contains. The virtual work done by viscous damping forces is given as WD = {u}T [Cdamp ]{u̇} dV , (9) V where [Cdamp ] is the proportional damping coefficient matrix and is expressed in terms of mass [M] and stiffness [K] matrices with the help of constants and as [Cdamp ] = [M] + [K]. (10) 4. Derivation of nonlinear FE equations The displacement field {u} and the electric potential at any point in a finite element are related to the corresponding nodal values {ui } and {i } by means of the element shape function matrices [Nu ] and [N ] as {u} = [Nu ]{ui } and = [N ]{i }, respectively. The strain field vector {S} and the electric field vector {E} can be expressed in terms of {ui } and {i } with the help of [Bu ] and [B ] as {S} = [Bu ]{ui } and {E} = [B ]{i }, where [Bu ] and [B ] are derivatives of shape function matrices. Incorporating these expressions of {S} and {E} into the variational equation (8), collecting the terms with {ui }T and {i }T and equating them to zero separately, we obtain the following coupled FE equations. [M]{ü} + [Cdamp ]{u̇} + [Kuu ]{ui } + [Ku ]{i } = {fi }, (11) [Ku ]{ui } + [K ]{i } = {gi }, (12) where [M] is the mass matrix, [Kuu ] is the nonlinear mechanical stiffness matrix, [Ku ] and [Ku ] are nonlinear piezoelectric stiffness matrices, [K ] is the nonlinear dielectric stiffness matrix, {fi } is 1470 the external mechanical force vector, and {gi } is the external electrical force vector respectively. The expressions for these matrices are given in Appendix-A1. It may be noted that the stiffness matrices are not constants. They depend implicitly upon the solution, i.e., {ui } and {i }. In order to assemble the element stiffness matrices, a special linearization technique (named Classical linearization after Salinas et al. [20]) has been adopted. In this technique, the initial solutions for {ui } and {i } are taken as the solutions of the corresponding linear equations. The matrices are then assembled and the global dynamic-coupled equations are solved using the Newmark- method after applying proper mechanical and electrical boundary conditions. In this way, the next approximate solution for the current time step is obtained. Again, the matrices are updated with the recent approximate solution and the method is repeated till the two consecutive solution vectors converge within a pre-specified tolerance limit. 5. Experimental work Experiments were conducted for studying the nonlinear behaviour of piezoceramic plates for the inplane mode of vibration. The piezoceramics were excited close to their resonance frequencies in two ways, i.e., sweep-up (SU) and sweep-down (SD). In SU the frequency was increased from a low to a high value past the natural frequency and in SD, the process was reversed. This was done to observe the jump phenomenon. The line diagram of the experimental set-up is shown in Fig. 2. The excitation and measurements have been done with the help of a gain-phase analyser (HewlettPackard HP 4194A). It sends the excitation signal to the piezoceramic through a power amplifier (Bruel and kjaer 2713). The dynamic response (velocity) signal is captured with the help of a laser vibrometer (Polytec). The laser vibrometer has two units (i.e., optic unit and electronic unit). The optic unit (OFV 508) supplies the laser signal to the piezoceramic as well as senses the reflected signal. The electronic unit Fig. 2. Experimental set-up for measuring the nonlinear dynamic response of the piezo-plate. 1471 Fig. 3. FFT of the time domain signal when the plate is excited at 1/3rd of the first natural frequency. then processes the signal from the optic unit and it is fed to the test channel of the gain phase analyzer. The input signal to the piezoceramic from the power amplifier is also supplied to the reference channel of the gain phase analyser which then compares the signal from the test channel with respect to the reference channel to determine the gain and the phase difference between the two signals. The two signals are also viewed in the digital oscilloscope (Yokogawa DL708E). The applied voltages are measured from the oscilloscope display. The displacement responses for various values of applied voltages are discussed in the next section on FE analysis. The Fast Fourier Transform (FFT) of the time domain response signal of piezoceramic has also been conducted. For this purpose, the piezoceramic is excited with the help of a signal generator (HewlettPackard HP 33120A) instead of the gain-phase analyser. Sinusoidal excitation with a particular frequency is set in the signal generator. The response signal is measured with the help of the laser vibrometer. The time domain signal is then picked in the digital oscilloscope with a predefined sampling rate, sampling time and record length of the data (which have been initially chosen in the oscilloscope settings). Then FFT analysis is performed on the time domain data to know the presence of signals of frequencies other than the excitation frequency. Fig. 3 shows the FFT analysis of the time domain signal of the laser vibrometer from the piezo-plate when it is excited at one-third of the first in-plane natural frequency. It can be seen from Fig. 3 that there are two distinct peaks observed in the frequency domain, i.e., one at the excitation frequency and the other at a frequency which is three times the excitation frequency. This gives evidence that cubic-type nonlinearity is dominant in the response of the piezo-plate. 6. FE analysis of in-pane vibration of a rectangular piezoelectric plate The procedure developed in this work has been implemented in an in-house FE program “NLPIEZO”. The program has been thoroughly tested using several case studies from the literature [21]. We present here the FE analysis of the nonlinear response behaviour of a piezoceramic plate. The plate analysed in this case is a rectangular plate of 70 mm length, 20 mm width and 4 mm thickness and is made up of PIC 181 supplied by “PI Ceramics”, Lederhose, Germany (www.piceramic.de) (Fig. 4a). 1472 Fig. 4. (a) Figure of the piezo-plate used in the investigation. (b) 2-D finite element mesh of one-quarter of the piezo-plate. Fig. 5. Variation of x-direction displacement in the first in-plane mode of oscillation of the plate. Fig. 6. Variation of y-direction displacement in the first in-plane mode of oscillation of the plate. The plate is polarized along the thickness direction. Sinusoidal electric voltages of different amplitudes are applied across the thickness. The first in-plane mode of the free–free vibration of the plate is along its length direction. The variation of displacements along x (length) and y (width) directions for the first mode are shown in Figs. 5 and 6, respectively. The amplitude of vibration is measured with the help of a 1473 W L Fig. 7. Symmetric boundary conditions used for the first mode of vibration. laser vibrometer, which is focused along the length onto one end of the plate. The vibrometer measures the velocity amplitude, which is converted into the displacement amplitude by dividing it with the applied circular frequency of excitation . A frequency sweep is applied near the first resonance frequency of the plate. It was observed that the frequency response path was not the same for the up-sweep (frequency is increased) and down-sweep (frequency is decreased) method of excitation (Fig. 1). The nonlinear softening behaviour and jump phenomena are clearly observed. This response behaviour of the plate has been calculated using the nonlinear FE program NLPIEZO. As the thickness of the plate is very small compared to other dimensions, a 2-D plane stress analysis has been carried out. One-fourth of the plane of the plate has been analysed because of symmetry of the first in-plane mode of vibration. The finite element mesh used for this study is shown in Fig. 4b. A 5 × 5 4-noded isoparametric FE mesh has been used. A mesh convergence study had been carried out beforehand to ensure that further refining of mesh size is not required to obtain convergence in solution. The mechanical boundary condition is applied at the symmetric planes of the plate (i.e., u1 = 0 at x = 0 and u2 = 0 at y = 0 where 1 and 2 refer to x and y directions, respectively (Fig. 7)). The electric boundary condition is simple because we are not modelling the thickness of the plate. Electric potential is applied across the thickness and the whole plane of the plate is coated with an electrode (i.e., is imposed). Hence, the electric field can be assumed to be constant in the plane perpendicular to the thickness of the plate and is given by electric potential per unit thickness with a negative sign. Because of the above electrical boundary conditions, only the equation for the actuator [i.e., Eq. (11)] needs to be solved. The electric potential applied serves as an external loading on the plate. The linear and nonlinear material property matrices have been taken from reference [21]. These material property matrices are usually obtained using optimization techniques. Analytical solutions for simple geometries are obtained using perturbation method of solution of nonlinear differential equations and by comparing analytical solutions with experimental ones, the parameters for a material are obtained. The details of this method are given elsewhere [22]. The damping values (proportional damping constants) have been calculated from the experimental results using the half-power method. The mass proportional damping constant is assumed as zero and hence the stiffness proportional constant is used as the damping parameter. The variation of the stiffness proportional damping constant with an electric field is shown in Fig. 11 (Appendix-A2). The material property matrices are given in Appendix-A2 where [S E ] is the compliance matrix at a constant electric field. 1474 7. Results and discussion Fig. 8 shows the comparison of the predicted and experimental nonlinear frequency response of the plate for both up and down frequency sweep. Here we will briefly describe the method used to obtain different responses by FEM in sweep-up and sweep-down conditions of excitation. For the sweep-up condition, the system is excited at a frequency lower than the resonance frequency away from the jump region. It may be noted that the nonlinear response has to be detained for each particular applied frequency of excitation at a time. Once the converged solution of the nonlinear system for a particular frequency is obtained, one needs to proceed to the next frequency of excitation. An initial guess solution for a particular frequency is obtained by solving the corresponding linear problem. This solution is used to calculate the nonlinear matrices and then the linearized system is solved to obtain the next approximate solution. The process is repeated in an iterative manner till convergence in the solution vector is achieved. For the sweep-up frequency method, the converged response of the previous frequency (lower value) is used as an initial guess for the next higher frequency of excitation instead of starting from the linear problem. For the sweep-down method, the converged response of previous higher frequency is used for the solution of the next lower frequency. In a nonlinear problem, there are multiple solutions for a particular input (frequency of excitation) especially in the jump region. The convergence to a particular solution depends upon the initial guess solution used and the solution attained is that which is closer to the guess solution. This property has been exploited in this analysis to predict the different sweep-up and sweep-down frequency response behaviour of the piezo-plate. It can be observed from Fig. 8 that the model is able to accurately predict the nonlinear response of the piezo-plate. In order to study the effect of different electric fields on the nonlinear response of the piezo-plate, experiments have been conducted at different excitation voltages (i.e., from 3 to 35 V). The FEM-calculated displacement responses per unit voltage near the first resonance frequency for both sweep-up and sweep-down modes are shown in Fig. 9 for 5, 10 and 30 V, respectively. Fig. 8. Comparison of FEM-predicted and experimental nonlinear response behaviour of the piezo- excited near the first resonance frequency with 30 V. 1475 Fig. 9. Variation of displacement amplitude with electric field for the piezo-plate excited near the first resonance frequency calculated by FEM. Fig. 10. Variation of displacement amplitude with electric field for the piezo-plate excited near the first resonance frequency. The results of FEM were very close to those of the experiments as evident in Fig. 8 for the applied potential of 30 V. It can be seen from Fig. 9 that the displacement amplitude per unit voltage reduces drastically as the electric field is increased. It can also be observed that there is a shift in the frequency of maximum amplitude towards the lower frequency region for both sweep-up and sweep-down modes of the experiment. It reflects a strong softening effect in the piezoceramic behaviour as the electric field is increased. The change or decrease in the frequency corresponding to the maximum amplitude is higher for higher electric fields. The variation of the calculated displacement amplitude from FEM for the whole range of electric fields (i.e., 3 to 35 V divided by the thickness of the piezo-plate) is shown in Fig. 10. It can be observed that a strong nonlinear relationship exists between the displacement amplitude and the applied electric field. 1476 This nonlinear piezoelectric behaviour model has tremendous applications in the design of ultrasonic piezomotors and other piezoelectric systems (such as machine cutters, resonators, etc.) where the piezo is excited near its resonance frequency in order to obtain maximum response. In ring-type ultrasonic piezomotors, the different modes of vibration of the piezo-ring are used to generate elliptical motion of the stator and this in turn is used to move the rotor through a friction layer between the stator and rotor. The torque–speed characteristics of the system depend upon the vibration behaviour of the piezo-ring and the friction material. The nonlinear vibration behaviour modelled in this work may prove to be very important and if not envisaged beforehand can affect the predicted performance of the system. Hence, this behaviour should be considered carefully while modelling the performance of a piezoelectric system for different applications. Fig. 8 shows that the maximum amplitude of vibration of the plate is not at the natural frequency of the plate, but at a frequency less than that. It means the material undergoes softening due to the applied electric field and it occurs when the plate is excited near the natural frequency. The natural frequency of a coupled electro-mechanical system not only depends upon the mechanical, piezoelectric and dielectric material properties, but also upon the mechanical and electrical boundary conditions imposed. This becomes clear when one considers the natural vibration of a piezo-plate with voltage-driven electrodes (short-circuited) and charge-driven electrodes (open-circuited), respectively. In case of voltage-driven electrodes, the electrical field has no effect on the mechanical stiffness of the system and the natural frequency of vibration is the same as that of a pure mechanical system. On the other hand, the natural frequency is increased for a charge-driven electrode. This is because of the application of an external electric field boundary condition (i.e., applied electric field is zero at the electrodes) for this problem. It may be noted that the application of natural electric boundary conditions (electric potential) decreases the stiffness of the system (i.e., softening effect). Electric potential is generated in a piezoelectric continuum due to mechanical strain. The distribution of mechanical strain depends upon the frequency of excitation. When the system is vibrating at a particular mode, the strain is maximum at the nodes and minimum at the antinodes. The formation of nodes and antinodes imposes natural electrical boundary conditions on the problem and hence it decreases the natural frequency of the system. This phenomenon is pronounced at high values of strain and hence is observed only when the system is excited near the resonance frequencies. Also, it has been experimentally observed that this phenomenon is more pronounced for lower modes. For higher modes, the effect of nonlinearity decreases. The system also behaves like a nonlinear spring-damper system in addition to the observed softening. This phenomenon can only be modelled using a nonlinear differential equation similar to Duffing’s equation for the continuum. The equation has to be linearized in order to obtain a starting solution and is then solved iteratively. In this way, the effective stiffness of the system becomes a function of field variables. The nonlinear stiffness coefficient for the system is negative and hence it captures the softening behaviour. The model developed in this work is also able to predict the jump phenomenon because of the characteristics of Duffing’s equation. 8. Conclusion In this work, a generalized nonlinear electric enthalpy density function incorporating higher order nonlinear terms (quadratic and cubic) in the energy expression of the coupled piezoelectric medium has been formulated. The scope of this formulation is to model the nonlinearities in a system whose 1477 governing equations are similar to a Duffing oscillator. These behaviours of a Duffing oscillator (i.e., jump phenomenon and dependence of resonance frequency on vibration amplitude) have been observed through experiments on piezoceramic plates and rod geometries under weak electric fields when excited near the resonance frequencies. This nonlinear electric enthalpy density function has been used to derive the coupled FE equations through variational formulation. These equations have been solved using the linearization technique. Experiments have been conducted on rectangular piezoceramic PIC 181 plates at different external electric fields to study and quantify its nonlinear are given vibration behaviour with electric potential applied across the thickness. The plate is excited with a sinusoidal voltage and then frequency sweeps are given near the first resonance frequency and the frequency response is calculated using the software NLPIEZO based on the FE formulation developed in this work. The calculated results for the nonlinear response of the piezo-plate matched closely with those of the experiment. The following conclusions can be drawn from the above study: • The maximum amplitude of vibration of the plate for this case is not at the natural frequency of the plate, but at a frequency less than that. It means that the material undergoes softening due to the applied electric field and it occurs when the plate is excited near its natural frequency. The reason for this is due to inherent imposition of natural electrical boundary conditions. • The system also behaves like a nonlinear spring-damper system in addition to the observed softening. This phenomenon can only be modelled using a nonlinear differential equation similar to Duffing’s equation for the continuum. • The model is able to predict the nonlinear response behaviour of the piezo-plate accurately. This generalized 3-D formulation is incorporated into the FE software NLPIEZO and hence, it can be used to model any piezoelectric system with complex geometry and boundary conditions. In future work, it will be used to model nonlinearities of an ultrasonic piezomotor and a piezo-beam system. Acknowledgements The first author sincerely acknowledges the financial support provided by DAAD (German Academic Exchange Service) for carrying out part of this research work at Technical University of Darmstadt, Germany. This work is supported by the Deutsche Forschungs Gemeinschaft vide research grant Ha1060/36. The first two authors gratefully acknowledge the support received from Aeronautics Research and Development Board and Department of Science and Technology, India. Appendix-A1 (Finite element matrices of the nonlinear piezoelectric continuum) [M] = [Nu ]T [Nu ] dV V [Kuu ] [Bu ]T [C][Bu ] + [Bu ]T [diag({S})][C21 ][diag({S})][Bu ] + 41 [Bu ]T [diag({S})][C22 ][diag({S 2 })][Bu ] + 43 [Bu ]T [diag({S 2 })][C22 ]T [Bu ] dV , = V + 13 [Bu ]T [C1 ][diag({S})][Bu ] + 23 [Bu ]T [diag({S})][C1 ]T [Bu ] 1478 [Ku ] [Bu ]T [C]T [d]T [B ] + [Bu ]T [diag({S})][11 ]T [B ] dV , + 1 [Bu ]T [12 ]T [diag({E})][B ] + [Bu ]T [diag({S 2 })][21 ]T [B ] = 2 V 1 T T T T 2 +[Bu ] [diag({S})][22 ] [diag({E})][B ] + 3 [Bu ] [23 ] [diag({E })][B ] [Ku ] = [Ku ]T , [K ] [B ]T [0 ][B ] + 13 [B ]T [1 ][diag({E})][B ] + 23 [B ]T [diag({E})][1 ]T [B ] + 1 [B ]T [21 ][diag({E 2 })][B ] + 3 [B ]T [diag({E 2 })][21 ]T [B ] =− 4 4 V T +[B ] [diag({E})][22 ][diag({E})][B ] × dV , [Cdamp ] = [M] + [Bu ]T [C][Bu ], V {fi } = [Nu ] [FV ] dV + T V {gi } = − As2 As1 [Nu ]T [FAs ] dAs + [Nu ]T [FP ], [N ]T dAs − [N ]T Q. Appendix-A2 (Material properties of PIC 181) 1.1600 −0.4070 −0.4996 0 0 0 0 0 0 −0.4070 1.1750 −0.4996 0 0 0 −11 2 −0.4996 −0.4996 1.4110 [S E ] = 10 m /N, 0 0 0 3.5330 0 0 0 0 0 0 3.5330 0 0 0 0 0 0 3.1640 0 0 0 0 3.89 0 [d] = 0 0 0 3.89 0 0 10−10 m/V, −1.148 −1.148 2.53 0 0 0 4.7000 2.7914 2.6525 0 0 0 0 0 0 2.7914 4.7000 2.6525 2.6525 2.6525 3.9978 0 0 0 16 [C21 ] = − 10 N/m2 . 0 0 0.8465 0 0 0 0 0 0 0 0.8465 0 0 0 0 0 0 0.9452 The other nonlinear material properties have a negligible effect and are assumed to be zero. The mass proportional damping constant is assumed to be zero. So, the stiffness proportional damping constant is taken as the damping parameter. The variation of the damping parameter with applied electric field is shown in Fig. 11. 1479 Fig. 11. Variation of stiffness-proportional damping constant with the applied electric field for the piezo-plate. References [1] E.F. 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