Study of Energetic Ion Generation from HighIntensity-Laser Dense-Plasma Interactions K. Flippoa, A. Maksimchuka, S. Banerjeea, K. Nasha, V. Wonga, T. Lina, K. Nemotob, V. Yu. Bychenkovc, Y. Sentokud, G. Mouroua, D. Umstadtera "FOCUS Center, University of Michigan, Ann Arbor, MI 48109-2099, USA b CRIEPI, 2-11-1, Iwado-kita, Komae-shi, Tokyo, 201-8511 Japan P. N. Lebedev Physics Institute, Russian Academy of Science, 117924 Moscow, Russia d Osaka University, Osaka Japan (Currently with GA, San Diego) C Abstract. We report on the characteristics of an ultrafast-laser driven proton beam from thinfilm targets. The difference in proton beam profiles, beam energies, and laser induced back ablation plumes between a dielectric (Mylar) and a conductor (aluminum) are discussed. Evidence for front-side acceleration and a method for beam manipulation are also presented. IONS FROM HIGH-INTENSITY-LASERS Since the discovery of forward accelerated protons and ions from high-intensitylaser thin-film interactions1'2'3, many groups have become interested in using these protons for a wide variety of applications, including: plasma diagnostics4, radiography5, radiation therapy6, radioisotope production7'8, fast ignition fusion9, table-top nuclear reactions10 and nuclear physics11, and even space propulsion12. For these proton beams to become usefully wide-spread their origin must first be carefully understood and then their characteristics controlled. In our previous experiments2 we used the second harmonic light from a T3 hybrid Ti:Sapph/Nd:Glass laser system producing 10TW. These initial experiments were limited to 2 J and 2xl018 W/cm2 due to non-linear effects in the doubling crystal. We observed that a collimated beam of protons, 40° in divergence, and up to 1.5 MeV could be accelerated forward through the target. The protons originate from a few tens to hundreds of Angstroms thick contamination layer on the surface of the target, consisting of mainly water vapor. In a subsequent experiment8 we observed, using 6 J of the laser's fundamental frequency, at intensities up to 5xl018 W/cm2, that a beam of up to 10 MeV was CP647, Advanced Accelerator Concepts: Tenth Workshop, edited by C. E. Clayton and P. Muggli © 2002 American Institute of Physics 0-7354-0102-0/02/$19.00 255 Mylar Mylar film film CD CD / Boron Boron sample sample Laser Laser Deuterons Deuterons l10 !l|B |!i HC 11 c n FIGURE FIGURE 1. 1. Setup Setup for for 10B(d,n)11C 10B(d,n)l 1C nuclear nuclear activation activationexperiments. experiments. possible. possible. We We also also showed showed that that the the majority majority of of protons protons in in our our experiments experiments originated originated from the front surface of the target through an experiment from the front surface of the target through an experiment involving involving nuclear nuclear activation. activation. The thin The experiment experiment pictured pictured in in Fig. Fig. 11 consisted consisted of of laying laying down down aa very very thin layer layer of of 10 10B was placed deuterated plastic over a thin (6 micron) Mylar film. A sample of deuterated plastic over a thin (6 micron) Mylar film. A sample of B was placed behind behind the the target target (in (in the the forward forward direction), direction), then then the the Mylar Mylar was was irradiated irradiated by by the the laser laser either the coated side or uncoated side facing the boron. Activation, via the either with with the coated side or uncoated side facing the boron. Activation, via the 10 11 reaction was irradiated. reaction 10B(d,n) B(d,n)HC, C, was was seen seen only only when when the the deuterated deuterated surface surface was irradiated. 13 14 The The front front surface surface acceleration acceleration was was explained explained by by vv ×x BB13 or or Brunel Brunei14 heating heating of of the the electrons electrons and and acceleration acceleration into into the the solid. solid. This This produces produces aa large large electrostatic electrostatic field field which which accelerates accelerates the the protons protons into into the the target. target. Ponderomotive Ponderomotive forces forces alone alone could could not not explain the needed electron temperatures for the observed proton energies assuming explain the needed electron temperatures for the observed proton energies assuming the = CZ λI , where Z is the the electrostatic electrostatic potential potential imparts imparts energy energy to to the the ions ions as as EEmax max= CZ-Jdl, where Z is the atomic number, λI is the product of the laser wavelength and atomic number, Al is the product of the laser wavelength and the the intensity, intensity, and and CC is is the the proportionality constant. proportionality constant. This This explanation explanation is is only only valid valid for for aa laser-solid laser-solid interaction interaction in in which which there there isis aa high high laser contrast between the foot of the pulse (pre-pulse) and the main laser contrast between the foot of the pulse (pre-pulse) and the main pulse. pulse. In In 7our our experiment experiment using using the the second second harmonic harmonic the the laser laser contrast contrast was was approximately approximately 10 107:1, :1, which which did did not not produce produce aa significant significant pre-plasma pre-plasma (1 (1 micron micron or or less), less), with with which which the the highest highest intensity intensity portion portion of of the the pulse pulse could could interact. interact. 5 However, However, experiments experiments at at the the fundamental fundamental frequency frequency had had aa contrast contrast of of only only 10 105:1, :1, and and aa pre-plasma pre-plasma from from several several to to ten ten microns microns could could form. form. The The formation formation of of the the prepreplasma plasma is is critical critical to to acceleration acceleration of of ions, ions, because because of of the the increase increase in in absorbed absorbed laser laser radiation. radiation. 2 Hatchet Hatchet et. et. al. al. and and Snavely Snavely et. et. al. al2 have have done done experiments experiments which which they they interpret interpret as as having protons which originated on the back surface, and in fact have shown via PIC having protons which originated on the back surface, and in fact have shown via PIC 15 simulation simulation15 that that both both surfaces surfaces produce produce protons. protons. Controlling Controlling which which surface surface produces produces the beam of protons may lead to applications for each method. the beam of protons may lead to applications for each method. 256 Protons CR-39 Protons Protons Laser Protons Protons Laser (a) Flat Flat (a) (b) Round Round (b) 100-120 micron diameter aluminum half-wire target results. Flat side (a) and round side FIGURE 2. 100-120 841 (b). (b). The The wires were oriented oriented (b) irradiated, protons are recorded on CR-39 numbered 840 (a) and 841 approximately 45 degrees to the vertical, indicated by dashed lines. Beam Manipulation Much theoretical work on methods to control proton/ion beam production has been introduced in the literature16. However, many of these methods require a precision in target control which is not yet achievable. We have taken the idea of micro shaped 100-150 microns targets to a macroscopic application. Using a half-wire of between 100-150 we observed an effect of the front surface on the produced beam. The laser focal spot 10 microns FWHM, with 40% of the total energy in that area. Fig. 2 was around 10 shows the results from the aluminum half-wire. the protons protons is is CR-39, CR-39, aa nuclear nuclear track track detector detector 22 xx 22 The detector used to record the inches in area, which is insensitive to x-rays or electrons. Fig. 2 shows the flat surface (a) produces a round beam on CR-39 similar to that of an ordinary flat thin-film target. The round surface (b), however, produces an uncollimated spray of protons on either side of the wire, as would be expected from the cylindrical lens-like surface defocusing the beam. Also, targets were made from 25 micron aluminum films, shaped to have different radii of curvature by different diameter ball bearings ranging from 0.4 to 11 mm in diameter. Fig. 3 shows the target geometry (on the left) with an inset image from the 0.2 mm radius target. The results of firing on the rounded side of two thin-film thin-film targets of 0.2 and 0.5 mm radii of curvature are shown on the right. CR-39 numbers 805 and 793 are beams produced from a target with a radius of 0.2 mm, and numbers 808 and 257 Laser Laser Laser >>1.2MeV 1.2 MeV MeV > 1.2 Protons Protons Target Target Holder Holder Holder CR-39 CR-39 1.8 MeV MeV >> 1.8 Target Target >>1.2 1.2 MeV » o »> 1 . 2 MeV M eV 2.5 MeV 2.5MeV MeV >>> 2.5 FIGURE 3. Left: Top view of the target geometry is shown, shown, inset inset of of slide slide 807 807 shows shows >> 1.8 1.8 MeV MeV for for FIGURE 3. Left: Top view of the target geometry is shown, inset of slide 807 shows > 1.8 MeV for radius. Right: CR-39 results are shown: 805 and 793 were produced from a 0.2 mm radius 0.2mm 0.2mm radius. Right: CR-39 results are shown: 805 and 793 were produced from a 0.2 mm radius target; 809 and 808 from aa 0.5 0.5 mm radius radius target. target. All All slides slides are are from from separate separate shots. shots. ttarget; arget; 809 and 808 from from a 0.5 mm mm radius target. All slides are from separate shots. mm radius radius target, target, though though each each slide slide isis is from from aaa 809 0.5 mm mm radius target, though each slide from 809 are are beams beams produced produced from from aaa 0.5 separate shot. It must be noted that the CR-39 images here are misleading. In fact separate shot. It must be noted that the CR-39 images here are misleading. In fact what appears to be a ring with a density depression on axis, is actually an what appears to be a ring with a density depression on axis, is actually an oversaturated region in the center and appears brighter due to overlapping tracks. CRoversaturated region in the center and appears brighter due to overlapping tracks. CR39 increasingly opaque with with increasing increasing track track density, density, until until itit saturates saturates (at (at 39 will will become become increasingly opaque 5 5 particles/mm22), then its opacity will decrease. Physical inspection under a aa few 10 few 10 particles/mm ), then its opacity will decrease. Physical inspection under a microscope myriad of tracks can be seen, the myriad of tracks can easily easily be seen, microscope reveals reveals the the dissimilarity; dissimilarity; the differentiating saturated differentiating it from regions of low track density. The saturated differentiating it from regions of low track density. The saturated area an area area of of increased increased flux, flux, which which is is not not seen seen in in aa typical typical area can can then then be be interpreted interpreted as as an beam 808 and 809. The from a flat target, or in the larger radius targets of slides 808 and 809. The beam from a flat target, or in the larger radius targets of slides 808 and 809. The radius the beam image being smaller target is harder to align, and this may account for smaller radius target is harder to align, and this may account for the beam image being off-center 1.8 off-center inset on on the the left left is is included included to to show show aa strong strong beam beam >> 1.8 1.8 off-center on on the the CR-39. CR-39. The The inset 19 19 22, here we see MeV the 0.2 mm radius at an intensity of nearly 2*10 W/cm from 2×10 MeV from the 0.2 mm radius at an intensity of nearly 2×10 W/cm , here we see "hole" in clearly in the the center, center, and and its its high high degree degree of of symmetry symmetry when when clearly the the high high flux flux “hole” “hole” properly properly aligned. aligned. (a) (b) tit* (c) (c) (c) £<§« 13 micron 12.5 micron FIGURE 13 micron Mylar Mylar (a) (a) and and 12.5 12.5 micron FIGURE 4. Images of beams on radiochromic film from 13 (c) from from that that same same shot. shot. aaluminum luminum (b) with a subsequent piece of CR-39 (c) aluminum 258 BEAMS FROM DIELECTRICS AND CONDUCTORS A real-time non-destructive diagnostic for the proton beam is being investigated. Currently we are looking at the plasma plume to gain insight into the proton beam's energy and spatial features. It has been noted that the beam quality varies greatly when using a dielectric versus a conductor. Fig 4 (a) elucidates the difference: a radiochromic film image of a beam from a 13 micron Mylar target, compared to that of (b) a 12.5 micron aluminum target. Radiochromic film has been shown by Clarke et. a/.1 that the signature of radiochromic film corresponds well with that of the proton beam, as can be seen from our results as well in Fig. 4 (b) and (c) in which a slide of CR-39 (c) was behind the Radiochromic film on the same shot. The Mylar shot (a) shows a remarkable star-like structure, where as the aluminum is fairly uniform. A similarly symmetric pattern is shown on CR-39 from different shot, and different beam energies in Fig 5. Fig. 5 shows the complicated beam structure which arises from a dielectric target (13 microns of Mylar), and the large difference as compared to the CR-39 in Fig. 4 (c), and also Fig. 3 (808), (809), which, as stated previously, have beam profiles nearly identical to those from flat target beams. The complex structure is thought to arise from huge (30MG) magnetic fields inside the dielectrics17. Not only is the beam quality different, but the maximum proton energies for Mylar and aluminum are about 2 times different. Fig. 6 shows the maximum proton energy versus material thickness for aluminum at the second harmonic (triangles), aluminum at the fundamental (squares), and Mylar at the fundamental (circles). Using the second harmonic of the laser the contrast is 3 orders of magnitude better, but the maximum proton energy is lower. This is due to the need for a certain scale length of pre-plasma before the main pulse arrives. This pre-plasma, created by the foot of the laser pulse, allows for a standing wave in the under dense plasma to heat the electrons, stochastically, to much hotter temperatures18, and thus yield hotter protons. The aluminum (triangles) at the second harmonic does not have a peak nor did material choice effect the maximum proton energy, unlike the Mylar (circles) and aluminum (squares) at the fundamental frequency of the laser which both have peaks around 1213 microns and show material dependence on proton energy. The solid line is a calculation taking into account the target thickness and accounting for the proton's > 1.2 MeV > 1.8 MeV > 2.5 MeV FIGURE 5. Beam images on CR-39 2 cm away from a 13 micron Mylar target from 1.2 to 2.5 MeV. 259 Proton Proton Energy Energy vs. vs. Target Target Thickness Thickness Max. Proton Energy[MeV] 14 12 A 10 Al Al Taget Taget @ @ 532 532 nm nm -A11111111111111 Al Al dE/dx dE/dx corrected corrected 8 m 6 Al Al Target Target @ @ 1.053 1.053 um um Al dE/dx -•—Al dE/dx corrected corrected 4 © 2 Mylar Mylar Target Target @1.053 @1.053 um um Mylar dE/dx «^^«My\ar dE/dx corrected corrected 0 00 50 50 100 100 150 150 Target Target Thickness Thickness [microns] [microns] 200 200 FIGURE FIGURE 6. 6. Maximum Maximum proton proton energy energy versus versus target target thickness thickness is is shown shown for for aluminum aluminum (triangles) (triangles) at at 18 19 2x10 2x1018 W/cm2, W/cm2, and and Mylar Mylar (circles); (circles); and and aluminum aluminum (squares) (squares) at at 11 xx 10 1019 W/cm2. W/cm2. Lines Lines are are the the calculated calculated energy energy loss loss (dE/dx) (dE/dx) correction correction values values for for protons protons having having traveled traveled through through the the target. target. energy energy loss loss (dE/dx) (dE/dx) through through the the material material with with the the assumption assumption all all originate originate on on the the front front surface. surface. ItIt is is easy easy to to see see that that the the protons protons from from the the front front surface surface appear appear to to saturate saturate and and plateau plateau at at about about 44 MeV MeV as as the the target target thickness thickness isis increased. increased. We We explain explain the the plateau plateau behavior behavior of of the the energy-loss energy-loss corrected corrected data data as as aa beam beam of of protons protons of of approximately approximately 44 MeV MeV produced produced at at the the front front surface surface of of the the target, target, propagating propagating through through the the target target and and losing losing energy energy proportional proportional to to the the distance distance they they travel travel through through the the aluminum aluminum target. target. 19 In report peak, only In contrast contrast to to the the observed observed peak peak Mackinnon Mackinnon et. et. al. al19 report seeing seeing no no peak, only aa steep steep decrease decrease in in proton proton energy energy followed followed by by aa much much gentler gentler decrease decrease as as the the thickness thickness increases. increases. The The steep steep decrease decrease is is explained explained by by electrons electrons recirculation recirculation inside inside the the target target during the during the the laser laser pulse pulse duration duration (100 (100 fs) fs) which which heats heats them them more more efficiently. efficiently. If If the target target is is too too thick thick (about (about 25 25 microns) microns) the the electrons electrons can can not not recalculate recalculate optimally optimally and and do do not not heat heat as as much, much, thus thus the the protons protons are are not not efficiently efficiently accelerated accelerated to to high high energies, energies, and and the the slope slope flattens flattens out. out. An An alternative alternative explanation explanation of of the the nature nature of of the the flattened flattened slope slope is is that that at at the the front front surface surface of of their their targets targets they they are are producing producing aa beam beam of of approximately approximately 8.5 8.5 MeV MeV protons protons due due to to the the approximately approximately 10 10 times times greater greater intensity. intensity. This This beam beam then then propagates propagates though though the the target, target, from from 20 20 to to 60 60 um um 8-9 8-9 MeV MeV protons protons would would lose lose only only between between 3-6% 3-6% of of their their initial initial energy, energy, and and at at 100 100 um um this this would would increase increase to to about about 15% 15% which which would would correspond correspond to to their their data data points. points. It It is is entirely entirely possible possible though though that that some some or or all all of of the the higher higher energy energy protons protons originate originate from from the the rear rear surface, surface, and and the the two two slopes slopes are are an an artifact artifact of of the the two two origins origins of of the the beams. beams. 260 PLUMES FROM DIELECTRICS AND CONDUCTORS Laser ablation plumes with longpulse (ns) lasers have been previously well studied theoretically20 and experimentally21 in the late 70's and 80's. When high power Chirped Pulse Amplified (CPA) picosecond and femtosecond lasers22 became widely available in the early 90 's solid target interactions and their associated plasma plumes began to be studied extensively both experimentally23 and theoretically24. In addition, when high-intensity subpicosecond lasers were used, superthermal ions were observed25, which are of great interest to the laser deposited materials community. However, the rear-side subpicosecond laser induced back ablation (LIBA) plume, has not been studied in any detail in the high-intensity regime. Some earlier work has been done at lower intensities with nanosecond pulses with thin films supported by transparent substrates26, and similar work has been done in the 35 picosecond regime27, but the plume itself was not the intended point of study. We report on the use of the plasma plume integrated optical emission as a diagnostic for thin film properties. The plasma plume geometry and intensity can be used to determine the relative strength of the laser coupling to the material as well as the type of material. The term LIBA can be a confusing term since the proton beam is FIGURE 7. Integrated optical plume images for aluminum (top) and Mylar (bottom) for various thicknesses. Plane of the target is out of the page, dashed line indicates target plane, laser is incident from the bottom. Imaged light is from 700nm - 350nm with a gap of 20 nm around 532 to block the second harmonic. 261 accelerated in in the forward forward direction, direction, hence hence we we shall shall refer refer to to itit as as the the forward forward directed directed accelerated ablation plume (FDAP). (FDAP). The The FDAP FDAP from from dielectric dielectric targets targets have have marked marked characteristic characteristic ablation differences from from that of of conductors. conductors. Fig. Fig. 77 shows shows the the FDAP FDAP from from aluminum aluminum (top) (top) and and differences Mylar (bottom) (bottom) targets. between the plumes plumes is is easy easy to to see, see, the the bright bright spot spot is is the the From Fig. 77 the difference between laser interaction interaction region, and and the white dashed dashed line line indicates indicates the the target target plane. plane. The The laser laser laser is incident incident from from the the bottom bottom of of the the dashed dashed line. line. The The aluminum aluminum (top) (top) shows shows aa uniform uniform is and rounded rounded top top structure. structure. The The Mylar Mylar plumes plumes (bottom) (bottom) plume with aa tree-like trunk and double lobe lobe feature feature in in the the expanding expanding plume, plume, with with aa dark dark region region between between have aa unique double and aa fan-like fan-like shape. shape. This This structure structure may may be be due due to to chemiluminesence chemiluminesence in in the two lobes, and of the beam as as carbon carbon oxidizes, oxidizes, however however similar similar structures structures have have been been the outer region of seen in in mostly hydrogen atmospheres. atmospheres. seen a b c d Intensity vs. vs. PIN PIN Diode Diode Output Output Intensity 3 PIN Diode Signal [V] 2.5 2.5 2 y = 0.028x - 0.7334 1.5 1.5 1 0.5 0.5 0 0 20 20 40 40 60 60 80 80 100 100 120 120 Peak Intensity Intensity [a.u.] [a.u.] Peak FIGURE FIGURE 8. 8. At At top are are 44 images images of of 13 13 micron micron Mylar Mylar plumes plumes (a-d) (a-d) at at various various PIN PIN diode diode signal signal voltages, voltages, 2.5V (a), (a), 2V 2V (b), (b), 0.75V 0.75V (c), (c), and and 0.5 0.5 V(d); V(d); the the graph graph below below shows shows the the correlation correlation between between the the PIN PIN diode diode voltage and and aa 40-line-averaged 40-line-averaged line line out out along along the the white white line. line. 262 A PIN diode is in the chamber to monitor the X-ray signal produced from the hot electrons. We, as well as Badziak28, have noted a correlation of the produced x-rays and the proton energy. X-rays are known to correlate with the hot-electron temperature29, and the hot-electrons, as discussed above, are responsible for ion acceleration. Thus x-ray PIN diode signals are a main diagnostic of the interaction. Now, however, we may have a new alternative. Figure 8 shows a set of plumes from 13 micron Mylar for various PIN diode voltages with a 40-line averaged line-out from the area of the plume below the lobed structure as indicated by the white line in Fig. 8. The intensity of this area correlates linearly with the PIN diode signal, which as stated above, correlates with the maximum proton energy. It is our hope that we can refine this technique and implement it as a real time beam diagnostic. SUMMARY We have shown that there exists a beam of protons from high-intensity laser interactions with thin-film targets which originates on the laser irradiated (front) side. We are able to control to some degree the beam by shaping the target's front surface. We have observed a difference in maximum proton energies for Mylar and aluminum, and a peak in the target thickness dependence. 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